Sensitivity of chemical tracers to meteorological parameters in the MOZART-3 chemical transport model
Identifieur interne : 000117 ( PascalFrancis/Corpus ); précédent : 000116; suivant : 000118Sensitivity of chemical tracers to meteorological parameters in the MOZART-3 chemical transport model
Auteurs : D. E. Kinnison ; G. P. Brasseur ; S. Walters ; R. R. Garcia ; D. R. Marsh ; F. Sassi ; V. L. Harvey ; C. E. Randall ; L. Emmons ; J. F. Lamarque ; P. Hess ; J. J. Orlando ; X. X. Tie ; W. Randel ; L. L. Pan ; A. Gettelman ; C. Granier ; T. Diehl ; U. Niemeier ; A. J. SimmonsSource :
- Journal of geophysical research [ 0148-0227 ] ; 2007.
Descripteurs français
- Pascal (Inist)
- Analyse sensibilité, Traceur chimique, Transport, Modèle climat, Ozone, Troposphère, Mésosphère, Champ météorologique, Atmosphère, Prévision météorologique, Réanalyse, Méthane, Vapeur eau, Azote minéral, Climatologie, Satellite, Age, Air, In situ, Vent, Température, Simulation, Stratosphère, Oscillation quasi biennale, Circulation.
English descriptors
- KwdEn :
- Climate models, Climatology, Inorganic nitrogen, Mesosphere, Meteorological field, Quasi biennial oscillation, Reanalysis, Weather forecast, age, air, atmosphere, chemical tracers, circulation, in situ, methane, ozone, satellites, sensitivity analysis, simulation, stratosphere, temperature, transport, troposphere, water vapor, winds.
Abstract
The Model for Ozone and Related Chemical Tracers, version 3 (MOZART-3), which represents the chemical and physical processes from the troposphere through the lower mesosphere, was used to evaluate the representation of long-lived tracers and ozone using three different meteorological fields. The meteorological fields are based on (1) the Whole Atmosphere Community Climate Model, version 1b (WACCMIb), (2) the European Centre for Medium-Range Weather Forecasts (ECMWF) operational analysis, and (3) a new reanalysis for year 2000 from ECMWF called EXP471. Model-derived tracers (methane, water vapor, and total inorganic nitrogen) and ozone are compared to data climatologies from satellites. Model mean age of air was also derived and compared to in situ CO2 and SF6 data. A detailed analysis of the chemical fields simulated by MOZART-3 shows that even though the general features characterizing the three dynamical sets are rather similar, slight differences in winds and temperature can produce substantial differences in the calculated distributions of chemical tracers. The MOZART-3 simulations that use meteorological fields from WACCMIb and ECMWF EXP471 represented best the distribution of long-lived tracers and mean age of air in the stratosphere. There was a significant improvement using the ECMWF EXP471 reanalysis data product over the ECMWF operational data product. The effect of the quasi-biennial oscillation circulation on long-lived tracers and ozone is examined.
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Format Inist (serveur)
| NO : | PASCAL 08-0011558 INIST |
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| ET : | Sensitivity of chemical tracers to meteorological parameters in the MOZART-3 chemical transport model |
| AU : | KINNISON (D. E.); BRASSEUR (G. P.); WALTERS (S.); GARCIA (R. R.); MARSH (D. R.); SASSI (F.); HARVEY (V. L.); RANDALL (C. E.); EMMONS (L.); LAMARQUE (J. F.); HESS (P.); ORLANDO (J. J.); TIE (X. X.); RANDEL (W.); PAN (L. L.); GETTELMAN (A.); GRANIER (C.); DIEHL (T.); NIEMEIER (U.); SIMMONS (A. J.) |
| AF : | National Center for Atmospheric Research/Boulder, Colorado/Etats-Unis (1 aut., 2 aut., 3 aut., 4 aut., 5 aut., 6 aut., 9 aut., 10 aut., 11 aut., 12 aut., 13 aut., 14 aut., 15 aut., 16 aut.); Laboratory for Atmospheric and Space Physics, University of Colorado/Boulder, Colorado/Etats-Unis (7 aut., 8 aut.); Aeronomy Laboratory, NOAA/Boulder, Colorado/Etats-Unis (17 aut.); Service d'Aéronomie, University of Paris 6/Paris/France (17 aut.); Goddard Earth Sciences and Technology Center, University of Maryland, Baltimore County/Baltimore, Maryland/Etats-Unis (18 aut.); Max Planck Institute for Meteorology/Hamburg/Allemagne (19 aut.); European Centre for Medium-Range Weather Forecasts/Reading/Royaume-Uni (20 aut.) |
| DT : | Publication en série; Niveau analytique |
| SO : | Journal of geophysical research; ISSN 0148-0227; Etats-Unis; Da. 2007; Vol. 112; No. D20; D20302.1-D20302.24; Bibl. 1 p.3/4 |
| LA : | Anglais |
| EA : | The Model for Ozone and Related Chemical Tracers, version 3 (MOZART-3), which represents the chemical and physical processes from the troposphere through the lower mesosphere, was used to evaluate the representation of long-lived tracers and ozone using three different meteorological fields. The meteorological fields are based on (1) the Whole Atmosphere Community Climate Model, version 1b (WACCMIb), (2) the European Centre for Medium-Range Weather Forecasts (ECMWF) operational analysis, and (3) a new reanalysis for year 2000 from ECMWF called EXP471. Model-derived tracers (methane, water vapor, and total inorganic nitrogen) and ozone are compared to data climatologies from satellites. Model mean age of air was also derived and compared to in situ CO2 and SF6 data. A detailed analysis of the chemical fields simulated by MOZART-3 shows that even though the general features characterizing the three dynamical sets are rather similar, slight differences in winds and temperature can produce substantial differences in the calculated distributions of chemical tracers. The MOZART-3 simulations that use meteorological fields from WACCMIb and ECMWF EXP471 represented best the distribution of long-lived tracers and mean age of air in the stratosphere. There was a significant improvement using the ECMWF EXP471 reanalysis data product over the ECMWF operational data product. The effect of the quasi-biennial oscillation circulation on long-lived tracers and ozone is examined. |
| CC : | 001E; 001E01; 220 |
| FD : | Analyse sensibilité; Traceur chimique; Transport; Modèle climat; Ozone; Troposphère; Mésosphère; Champ météorologique; Atmosphère; Prévision météorologique; Réanalyse; Méthane; Vapeur eau; Azote minéral; Climatologie; Satellite; Age; Air; In situ; Vent; Température; Simulation; Stratosphère; Oscillation quasi biennale; Circulation |
| ED : | sensitivity analysis; chemical tracers; transport; Climate models; ozone; troposphere; Mesosphere; Meteorological field; atmosphere; Weather forecast; Reanalysis; methane; water vapor; Inorganic nitrogen; Climatology; satellites; age; air; in situ; winds; temperature; simulation; stratosphere; Quasi biennial oscillation; circulation |
| SD : | Transporte; Ozono; Mesosfera; Campo meteorológico; Atmósfera; Predicción meteorológica; Reánalisis; Metano; Vapor agua; Nitrógeno inorgánico; Climatología; Satélite; Edad; Viento; Temperatura; Simulación; Estratosfera; Oscilación cuasi bienal |
| LO : | INIST-3144.354000173593090370 |
| ID : | 08-0011558 |
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Pascal:08-0011558Le document en format XML
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Diehl</name><affiliation><inist:fA14 i1="05"><s1>Goddard Earth Sciences and Technology Center, University of Maryland, Baltimore County</s1><s2>Baltimore, Maryland</s2><s3>USA</s3><sZ>18 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Niemeier, U" sort="Niemeier, U" uniqKey="Niemeier U" first="U." last="Niemeier">U. Niemeier</name><affiliation><inist:fA14 i1="06"><s1>Max Planck Institute for Meteorology</s1><s2>Hamburg</s2><s3>DEU</s3><sZ>19 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Simmons, A J" sort="Simmons, A J" uniqKey="Simmons A" first="A. J." last="Simmons">A. J. Simmons</name><affiliation><inist:fA14 i1="07"><s1>European Centre for Medium-Range Weather Forecasts</s1><s2>Reading</s2><s3>GBR</s3><sZ>20 aut.</sZ></inist:fA14></affiliation></author></titleStmt><publicationStmt><idno type="wicri:source">INIST</idno><idno type="inist">08-0011558</idno><date when="2007">2007</date><idno type="stanalyst">PASCAL 08-0011558 INIST</idno><idno type="RBID">Pascal:08-0011558</idno><idno type="wicri:Area/PascalFrancis/Corpus">000117</idno></publicationStmt><sourceDesc><biblStruct><analytic><title xml:lang="en" level="a">Sensitivity of chemical tracers to meteorological parameters in the MOZART-3 chemical transport model</title><author><name sortKey="Kinnison, D E" sort="Kinnison, D E" uniqKey="Kinnison D" first="D. E." last="Kinnison">D. E. Kinnison</name><affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ><sZ>9 aut.</sZ><sZ>10 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>14 aut.</sZ><sZ>15 aut.</sZ><sZ>16 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Brasseur, G P" sort="Brasseur, G P" uniqKey="Brasseur G" first="G. P." last="Brasseur">G. P. Brasseur</name><affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ><sZ>9 aut.</sZ><sZ>10 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>14 aut.</sZ><sZ>15 aut.</sZ><sZ>16 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Walters, S" sort="Walters, S" uniqKey="Walters S" first="S." last="Walters">S. Walters</name><affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ><sZ>9 aut.</sZ><sZ>10 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>14 aut.</sZ><sZ>15 aut.</sZ><sZ>16 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Garcia, R R" sort="Garcia, R R" uniqKey="Garcia R" first="R. R." last="Garcia">R. R. Garcia</name><affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ><sZ>9 aut.</sZ><sZ>10 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>14 aut.</sZ><sZ>15 aut.</sZ><sZ>16 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Marsh, D R" sort="Marsh, D R" uniqKey="Marsh D" first="D. R." last="Marsh">D. R. Marsh</name><affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ><sZ>9 aut.</sZ><sZ>10 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>14 aut.</sZ><sZ>15 aut.</sZ><sZ>16 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Sassi, F" sort="Sassi, F" uniqKey="Sassi F" first="F." last="Sassi">F. Sassi</name><affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ><sZ>9 aut.</sZ><sZ>10 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>14 aut.</sZ><sZ>15 aut.</sZ><sZ>16 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Harvey, V L" sort="Harvey, V L" uniqKey="Harvey V" first="V. L." last="Harvey">V. L. Harvey</name><affiliation><inist:fA14 i1="02"><s1>Laboratory for Atmospheric and Space Physics, University of Colorado</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>7 aut.</sZ><sZ>8 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Randall, C E" sort="Randall, C E" uniqKey="Randall C" first="C. E." last="Randall">C. E. Randall</name><affiliation><inist:fA14 i1="02"><s1>Laboratory for Atmospheric and Space Physics, University of Colorado</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>7 aut.</sZ><sZ>8 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Emmons, L" sort="Emmons, L" uniqKey="Emmons L" first="L." last="Emmons">L. Emmons</name><affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ><sZ>9 aut.</sZ><sZ>10 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>14 aut.</sZ><sZ>15 aut.</sZ><sZ>16 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Lamarque, J F" sort="Lamarque, J F" uniqKey="Lamarque J" first="J. F." last="Lamarque">J. F. Lamarque</name><affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ><sZ>9 aut.</sZ><sZ>10 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>14 aut.</sZ><sZ>15 aut.</sZ><sZ>16 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Hess, P" sort="Hess, P" uniqKey="Hess P" first="P." last="Hess">P. Hess</name><affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ><sZ>9 aut.</sZ><sZ>10 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>14 aut.</sZ><sZ>15 aut.</sZ><sZ>16 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Orlando, J J" sort="Orlando, J J" uniqKey="Orlando J" first="J. J." last="Orlando">J. J. Orlando</name><affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ><sZ>9 aut.</sZ><sZ>10 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>14 aut.</sZ><sZ>15 aut.</sZ><sZ>16 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Tie, X X" sort="Tie, X X" uniqKey="Tie X" first="X. X." last="Tie">X. X. Tie</name><affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ><sZ>9 aut.</sZ><sZ>10 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>14 aut.</sZ><sZ>15 aut.</sZ><sZ>16 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Randel, W" sort="Randel, W" uniqKey="Randel W" first="W." last="Randel">W. Randel</name><affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ><sZ>9 aut.</sZ><sZ>10 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>14 aut.</sZ><sZ>15 aut.</sZ><sZ>16 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Pan, L L" sort="Pan, L L" uniqKey="Pan L" first="L. L." last="Pan">L. L. Pan</name><affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ><sZ>9 aut.</sZ><sZ>10 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>14 aut.</sZ><sZ>15 aut.</sZ><sZ>16 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Gettelman, A" sort="Gettelman, A" uniqKey="Gettelman A" first="A." last="Gettelman">A. Gettelman</name><affiliation><inist:fA14 i1="01"><s1>National Center for Atmospheric Research</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ><sZ>9 aut.</sZ><sZ>10 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>14 aut.</sZ><sZ>15 aut.</sZ><sZ>16 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Granier, C" sort="Granier, C" uniqKey="Granier C" first="C." last="Granier">C. Granier</name><affiliation><inist:fA14 i1="03"><s1>Aeronomy Laboratory, NOAA</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>17 aut.</sZ></inist:fA14></affiliation><affiliation><inist:fA14 i1="04"><s1>Service d'Aéronomie, University of Paris 6</s1><s2>Paris</s2><s3>FRA</s3><sZ>17 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Diehl, T" sort="Diehl, T" uniqKey="Diehl T" first="T." last="Diehl">T. Diehl</name><affiliation><inist:fA14 i1="05"><s1>Goddard Earth Sciences and Technology Center, University of Maryland, Baltimore County</s1><s2>Baltimore, Maryland</s2><s3>USA</s3><sZ>18 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Niemeier, U" sort="Niemeier, U" uniqKey="Niemeier U" first="U." last="Niemeier">U. Niemeier</name><affiliation><inist:fA14 i1="06"><s1>Max Planck Institute for Meteorology</s1><s2>Hamburg</s2><s3>DEU</s3><sZ>19 aut.</sZ></inist:fA14></affiliation></author><author><name sortKey="Simmons, A J" sort="Simmons, A J" uniqKey="Simmons A" first="A. J." last="Simmons">A. J. Simmons</name><affiliation><inist:fA14 i1="07"><s1>European Centre for Medium-Range Weather Forecasts</s1><s2>Reading</s2><s3>GBR</s3><sZ>20 aut.</sZ></inist:fA14></affiliation></author></analytic><series><title level="j" type="main">Journal of geophysical research</title><title level="j" type="abbreviated">J. geophys. res.</title><idno type="ISSN">0148-0227</idno><imprint><date when="2007">2007</date></imprint></series></biblStruct></sourceDesc><seriesStmt><title level="j" type="main">Journal of geophysical research</title><title level="j" type="abbreviated">J. geophys. res.</title><idno type="ISSN">0148-0227</idno></seriesStmt></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Climate models</term><term>Climatology</term><term>Inorganic nitrogen</term><term>Mesosphere</term><term>Meteorological field</term><term>Quasi biennial oscillation</term><term>Reanalysis</term><term>Weather forecast</term><term>age</term><term>air</term><term>atmosphere</term><term>chemical tracers</term><term>circulation</term><term>in situ</term><term>methane</term><term>ozone</term><term>satellites</term><term>sensitivity analysis</term><term>simulation</term><term>stratosphere</term><term>temperature</term><term>transport</term><term>troposphere</term><term>water vapor</term><term>winds</term></keywords><keywords scheme="Pascal" xml:lang="fr"><term>Analyse sensibilité</term><term>Traceur chimique</term><term>Transport</term><term>Modèle climat</term><term>Ozone</term><term>Troposphère</term><term>Mésosphère</term><term>Champ météorologique</term><term>Atmosphère</term><term>Prévision météorologique</term><term>Réanalyse</term><term>Méthane</term><term>Vapeur eau</term><term>Azote minéral</term><term>Climatologie</term><term>Satellite</term><term>Age</term><term>Air</term><term>In situ</term><term>Vent</term><term>Température</term><term>Simulation</term><term>Stratosphère</term><term>Oscillation quasi biennale</term><term>Circulation</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">The Model for Ozone and Related Chemical Tracers, version 3 (MOZART-3), which represents the chemical and physical processes from the troposphere through the lower mesosphere, was used to evaluate the representation of long-lived tracers and ozone using three different meteorological fields. The meteorological fields are based on (1) the Whole Atmosphere Community Climate Model, version 1b (WACCMIb), (2) the European Centre for Medium-Range Weather Forecasts (ECMWF) operational analysis, and (3) a new reanalysis for year 2000 from ECMWF called EXP471. Model-derived tracers (methane, water vapor, and total inorganic nitrogen) and ozone are compared to data climatologies from satellites. Model mean age of air was also derived and compared to in situ CO<sub>2</sub> and SF<sub>6</sub> data. A detailed analysis of the chemical fields simulated by MOZART-3 shows that even though the general features characterizing the three dynamical sets are rather similar, slight differences in winds and temperature can produce substantial differences in the calculated distributions of chemical tracers. The MOZART-3 simulations that use meteorological fields from WACCMIb and ECMWF EXP471 represented best the distribution of long-lived tracers and mean age of air in the stratosphere. There was a significant improvement using the ECMWF EXP471 reanalysis data product over the ECMWF operational data product. The effect of the quasi-biennial oscillation circulation on long-lived tracers and ozone is examined.</div></front></TEI><inist><standard h6="B"><pA><fA01 i1="01" i2="1"><s0>0148-0227</s0></fA01><fA03 i2="1"><s0>J. geophys. res.</s0></fA03><fA05><s2>112</s2></fA05><fA06><s2>D20</s2></fA06><fA08 i1="01" i2="1" l="ENG"><s1>Sensitivity of chemical tracers to meteorological parameters in the MOZART-3 chemical transport model</s1></fA08><fA11 i1="01" i2="1"><s1>KINNISON (D. E.)</s1></fA11><fA11 i1="02" i2="1"><s1>BRASSEUR (G. P.)</s1></fA11><fA11 i1="03" i2="1"><s1>WALTERS (S.)</s1></fA11><fA11 i1="04" i2="1"><s1>GARCIA (R. R.)</s1></fA11><fA11 i1="05" i2="1"><s1>MARSH (D. R.)</s1></fA11><fA11 i1="06" i2="1"><s1>SASSI (F.)</s1></fA11><fA11 i1="07" i2="1"><s1>HARVEY (V. L.)</s1></fA11><fA11 i1="08" i2="1"><s1>RANDALL (C. E.)</s1></fA11><fA11 i1="09" i2="1"><s1>EMMONS (L.)</s1></fA11><fA11 i1="10" i2="1"><s1>LAMARQUE (J. F.)</s1></fA11><fA11 i1="11" i2="1"><s1>HESS (P.)</s1></fA11><fA11 i1="12" i2="1"><s1>ORLANDO (J. J.)</s1></fA11><fA11 i1="13" i2="1"><s1>TIE (X. X.)</s1></fA11><fA11 i1="14" i2="1"><s1>RANDEL (W.)</s1></fA11><fA11 i1="15" i2="1"><s1>PAN (L. L.)</s1></fA11><fA11 i1="16" i2="1"><s1>GETTELMAN (A.)</s1></fA11><fA11 i1="17" i2="1"><s1>GRANIER (C.)</s1></fA11><fA11 i1="18" i2="1"><s1>DIEHL (T.)</s1></fA11><fA11 i1="19" i2="1"><s1>NIEMEIER (U.)</s1></fA11><fA11 i1="20" i2="1"><s1>SIMMONS (A. J.)</s1></fA11><fA14 i1="01"><s1>National Center for Atmospheric Research</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>1 aut.</sZ><sZ>2 aut.</sZ><sZ>3 aut.</sZ><sZ>4 aut.</sZ><sZ>5 aut.</sZ><sZ>6 aut.</sZ><sZ>9 aut.</sZ><sZ>10 aut.</sZ><sZ>11 aut.</sZ><sZ>12 aut.</sZ><sZ>13 aut.</sZ><sZ>14 aut.</sZ><sZ>15 aut.</sZ><sZ>16 aut.</sZ></fA14><fA14 i1="02"><s1>Laboratory for Atmospheric and Space Physics, University of Colorado</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>7 aut.</sZ><sZ>8 aut.</sZ></fA14><fA14 i1="03"><s1>Aeronomy Laboratory, NOAA</s1><s2>Boulder, Colorado</s2><s3>USA</s3><sZ>17 aut.</sZ></fA14><fA14 i1="04"><s1>Service d'Aéronomie, University of Paris 6</s1><s2>Paris</s2><s3>FRA</s3><sZ>17 aut.</sZ></fA14><fA14 i1="05"><s1>Goddard Earth Sciences and Technology Center, University of Maryland, Baltimore County</s1><s2>Baltimore, Maryland</s2><s3>USA</s3><sZ>18 aut.</sZ></fA14><fA14 i1="06"><s1>Max Planck Institute for Meteorology</s1><s2>Hamburg</s2><s3>DEU</s3><sZ>19 aut.</sZ></fA14><fA14 i1="07"><s1>European Centre for Medium-Range Weather Forecasts</s1><s2>Reading</s2><s3>GBR</s3><sZ>20 aut.</sZ></fA14><fA20><s2>D20302.1-D20302.24</s2></fA20><fA21><s1>2007</s1></fA21><fA23 i1="01"><s0>ENG</s0></fA23><fA43 i1="01"><s1>INIST</s1><s2>3144</s2><s5>354000173593090370</s5></fA43><fA44><s0>0000</s0><s1>© 2008 INIST-CNRS. All rights reserved.</s1></fA44><fA45><s0>1 p.3/4</s0></fA45><fA47 i1="01" i2="1"><s0>08-0011558</s0></fA47><fA60><s1>P</s1></fA60><fA61><s0>A</s0></fA61><fA64 i1="01" i2="1"><s0>Journal of geophysical research</s0></fA64><fA66 i1="01"><s0>USA</s0></fA66><fC01 i1="01" l="ENG"><s0>The Model for Ozone and Related Chemical Tracers, version 3 (MOZART-3), which represents the chemical and physical processes from the troposphere through the lower mesosphere, was used to evaluate the representation of long-lived tracers and ozone using three different meteorological fields. The meteorological fields are based on (1) the Whole Atmosphere Community Climate Model, version 1b (WACCMIb), (2) the European Centre for Medium-Range Weather Forecasts (ECMWF) operational analysis, and (3) a new reanalysis for year 2000 from ECMWF called EXP471. Model-derived tracers (methane, water vapor, and total inorganic nitrogen) and ozone are compared to data climatologies from satellites. Model mean age of air was also derived and compared to in situ CO<sub>2</sub> and SF<sub>6</sub> data. A detailed analysis of the chemical fields simulated by MOZART-3 shows that even though the general features characterizing the three dynamical sets are rather similar, slight differences in winds and temperature can produce substantial differences in the calculated distributions of chemical tracers. The MOZART-3 simulations that use meteorological fields from WACCMIb and ECMWF EXP471 represented best the distribution of long-lived tracers and mean age of air in the stratosphere. There was a significant improvement using the ECMWF EXP471 reanalysis data product over the ECMWF operational data product. The effect of the quasi-biennial oscillation circulation on long-lived tracers and ozone is examined.</s0></fC01><fC02 i1="01" i2="3"><s0>001E</s0></fC02><fC02 i1="02" i2="2"><s0>001E01</s0></fC02><fC02 i1="03" i2="2"><s0>220</s0></fC02><fC03 i1="01" i2="2" l="FRE"><s0>Analyse sensibilité</s0><s5>01</s5></fC03><fC03 i1="01" i2="2" l="ENG"><s0>sensitivity analysis</s0><s5>01</s5></fC03><fC03 i1="02" i2="2" l="FRE"><s0>Traceur chimique</s0><s5>02</s5></fC03><fC03 i1="02" i2="2" l="ENG"><s0>chemical tracers</s0><s5>02</s5></fC03><fC03 i1="03" i2="2" l="FRE"><s0>Transport</s0><s5>03</s5></fC03><fC03 i1="03" i2="2" l="ENG"><s0>transport</s0><s5>03</s5></fC03><fC03 i1="03" i2="2" l="SPA"><s0>Transporte</s0><s5>03</s5></fC03><fC03 i1="04" i2="3" l="FRE"><s0>Modèle climat</s0><s5>04</s5></fC03><fC03 i1="04" i2="3" l="ENG"><s0>Climate models</s0><s5>04</s5></fC03><fC03 i1="05" i2="2" l="FRE"><s0>Ozone</s0><s5>05</s5></fC03><fC03 i1="05" i2="2" l="ENG"><s0>ozone</s0><s5>05</s5></fC03><fC03 i1="05" i2="2" l="SPA"><s0>Ozono</s0><s5>05</s5></fC03><fC03 i1="06" i2="2" l="FRE"><s0>Troposphère</s0><s5>06</s5></fC03><fC03 i1="06" i2="2" l="ENG"><s0>troposphere</s0><s5>06</s5></fC03><fC03 i1="07" i2="X" l="FRE"><s0>Mésosphère</s0><s5>07</s5></fC03><fC03 i1="07" i2="X" l="ENG"><s0>Mesosphere</s0><s5>07</s5></fC03><fC03 i1="07" i2="X" l="SPA"><s0>Mesosfera</s0><s5>07</s5></fC03><fC03 i1="08" i2="X" l="FRE"><s0>Champ météorologique</s0><s5>08</s5></fC03><fC03 i1="08" i2="X" l="ENG"><s0>Meteorological field</s0><s5>08</s5></fC03><fC03 i1="08" i2="X" l="SPA"><s0>Campo meteorológico</s0><s5>08</s5></fC03><fC03 i1="09" i2="2" l="FRE"><s0>Atmosphère</s0><s5>09</s5></fC03><fC03 i1="09" i2="2" l="ENG"><s0>atmosphere</s0><s5>09</s5></fC03><fC03 i1="09" i2="2" l="SPA"><s0>Atmósfera</s0><s5>09</s5></fC03><fC03 i1="10" i2="X" l="FRE"><s0>Prévision météorologique</s0><s5>10</s5></fC03><fC03 i1="10" i2="X" l="ENG"><s0>Weather forecast</s0><s5>10</s5></fC03><fC03 i1="10" i2="X" l="SPA"><s0>Predicción meteorológica</s0><s5>10</s5></fC03><fC03 i1="11" i2="X" l="FRE"><s0>Réanalyse</s0><s5>11</s5></fC03><fC03 i1="11" i2="X" l="ENG"><s0>Reanalysis</s0><s5>11</s5></fC03><fC03 i1="11" i2="X" l="SPA"><s0>Reánalisis</s0><s5>11</s5></fC03><fC03 i1="12" i2="2" l="FRE"><s0>Méthane</s0><s5>12</s5></fC03><fC03 i1="12" i2="2" l="ENG"><s0>methane</s0><s5>12</s5></fC03><fC03 i1="12" i2="2" l="SPA"><s0>Metano</s0><s5>12</s5></fC03><fC03 i1="13" i2="2" l="FRE"><s0>Vapeur eau</s0><s5>13</s5></fC03><fC03 i1="13" i2="2" l="ENG"><s0>water vapor</s0><s5>13</s5></fC03><fC03 i1="13" i2="2" l="SPA"><s0>Vapor agua</s0><s5>13</s5></fC03><fC03 i1="14" i2="X" l="FRE"><s0>Azote minéral</s0><s2>NK</s2><s5>14</s5></fC03><fC03 i1="14" i2="X" l="ENG"><s0>Inorganic nitrogen</s0><s2>NK</s2><s5>14</s5></fC03><fC03 i1="14" i2="X" l="SPA"><s0>Nitrógeno inorgánico</s0><s2>NK</s2><s5>14</s5></fC03><fC03 i1="15" i2="X" l="FRE"><s0>Climatologie</s0><s5>15</s5></fC03><fC03 i1="15" i2="X" l="ENG"><s0>Climatology</s0><s5>15</s5></fC03><fC03 i1="15" i2="X" l="SPA"><s0>Climatología</s0><s5>15</s5></fC03><fC03 i1="16" i2="2" l="FRE"><s0>Satellite</s0><s5>16</s5></fC03><fC03 i1="16" i2="2" l="ENG"><s0>satellites</s0><s5>16</s5></fC03><fC03 i1="16" i2="2" l="SPA"><s0>Satélite</s0><s5>16</s5></fC03><fC03 i1="17" i2="2" l="FRE"><s0>Age</s0><s5>17</s5></fC03><fC03 i1="17" i2="2" l="ENG"><s0>age</s0><s5>17</s5></fC03><fC03 i1="17" i2="2" l="SPA"><s0>Edad</s0><s5>17</s5></fC03><fC03 i1="18" i2="2" l="FRE"><s0>Air</s0><s5>18</s5></fC03><fC03 i1="18" i2="2" l="ENG"><s0>air</s0><s5>18</s5></fC03><fC03 i1="19" i2="2" l="FRE"><s0>In situ</s0><s5>19</s5></fC03><fC03 i1="19" i2="2" l="ENG"><s0>in situ</s0><s5>19</s5></fC03><fC03 i1="20" i2="2" l="FRE"><s0>Vent</s0><s5>20</s5></fC03><fC03 i1="20" i2="2" l="ENG"><s0>winds</s0><s5>20</s5></fC03><fC03 i1="20" i2="2" l="SPA"><s0>Viento</s0><s5>20</s5></fC03><fC03 i1="21" i2="2" l="FRE"><s0>Température</s0><s5>21</s5></fC03><fC03 i1="21" i2="2" l="ENG"><s0>temperature</s0><s5>21</s5></fC03><fC03 i1="21" i2="2" l="SPA"><s0>Temperatura</s0><s5>21</s5></fC03><fC03 i1="22" i2="2" l="FRE"><s0>Simulation</s0><s5>22</s5></fC03><fC03 i1="22" i2="2" l="ENG"><s0>simulation</s0><s5>22</s5></fC03><fC03 i1="22" i2="2" l="SPA"><s0>Simulación</s0><s5>22</s5></fC03><fC03 i1="23" i2="2" l="FRE"><s0>Stratosphère</s0><s5>23</s5></fC03><fC03 i1="23" i2="2" l="ENG"><s0>stratosphere</s0><s5>23</s5></fC03><fC03 i1="23" i2="2" l="SPA"><s0>Estratosfera</s0><s5>23</s5></fC03><fC03 i1="24" i2="X" l="FRE"><s0>Oscillation quasi biennale</s0><s5>24</s5></fC03><fC03 i1="24" i2="X" l="ENG"><s0>Quasi biennial oscillation</s0><s5>24</s5></fC03><fC03 i1="24" i2="X" l="SPA"><s0>Oscilación cuasi bienal</s0><s5>24</s5></fC03><fC03 i1="25" i2="2" l="FRE"><s0>Circulation</s0><s5>25</s5></fC03><fC03 i1="25" i2="2" l="ENG"><s0>circulation</s0><s5>25</s5></fC03><fN21><s1>007</s1></fN21><fN44 i1="01"><s1>OTO</s1></fN44><fN82><s1>OTO</s1></fN82></pA></standard><server><NO>PASCAL 08-0011558 INIST</NO><ET>Sensitivity of chemical tracers to meteorological parameters in the MOZART-3 chemical transport model</ET><AU>KINNISON (D. E.); BRASSEUR (G. P.); WALTERS (S.); GARCIA (R. R.); MARSH (D. R.); SASSI (F.); HARVEY (V. L.); RANDALL (C. E.); EMMONS (L.); LAMARQUE (J. F.); HESS (P.); ORLANDO (J. J.); TIE (X. X.); RANDEL (W.); PAN (L. L.); GETTELMAN (A.); GRANIER (C.); DIEHL (T.); NIEMEIER (U.); SIMMONS (A. J.)</AU><AF>National Center for Atmospheric Research/Boulder, Colorado/Etats-Unis (1 aut., 2 aut., 3 aut., 4 aut., 5 aut., 6 aut., 9 aut., 10 aut., 11 aut., 12 aut., 13 aut., 14 aut., 15 aut., 16 aut.); Laboratory for Atmospheric and Space Physics, University of Colorado/Boulder, Colorado/Etats-Unis (7 aut., 8 aut.); Aeronomy Laboratory, NOAA/Boulder, Colorado/Etats-Unis (17 aut.); Service d'Aéronomie, University of Paris 6/Paris/France (17 aut.); Goddard Earth Sciences and Technology Center, University of Maryland, Baltimore County/Baltimore, Maryland/Etats-Unis (18 aut.); Max Planck Institute for Meteorology/Hamburg/Allemagne (19 aut.); European Centre for Medium-Range Weather Forecasts/Reading/Royaume-Uni (20 aut.)</AF><DT>Publication en série; Niveau analytique</DT><SO>Journal of geophysical research; ISSN 0148-0227; Etats-Unis; Da. 2007; Vol. 112; No. D20; D20302.1-D20302.24; Bibl. 1 p.3/4</SO><LA>Anglais</LA><EA>The Model for Ozone and Related Chemical Tracers, version 3 (MOZART-3), which represents the chemical and physical processes from the troposphere through the lower mesosphere, was used to evaluate the representation of long-lived tracers and ozone using three different meteorological fields. The meteorological fields are based on (1) the Whole Atmosphere Community Climate Model, version 1b (WACCMIb), (2) the European Centre for Medium-Range Weather Forecasts (ECMWF) operational analysis, and (3) a new reanalysis for year 2000 from ECMWF called EXP471. Model-derived tracers (methane, water vapor, and total inorganic nitrogen) and ozone are compared to data climatologies from satellites. Model mean age of air was also derived and compared to in situ CO<sub>2</sub> and SF<sub>6</sub> data. A detailed analysis of the chemical fields simulated by MOZART-3 shows that even though the general features characterizing the three dynamical sets are rather similar, slight differences in winds and temperature can produce substantial differences in the calculated distributions of chemical tracers. The MOZART-3 simulations that use meteorological fields from WACCMIb and ECMWF EXP471 represented best the distribution of long-lived tracers and mean age of air in the stratosphere. There was a significant improvement using the ECMWF EXP471 reanalysis data product over the ECMWF operational data product. The effect of the quasi-biennial oscillation circulation on long-lived tracers and ozone is examined.</EA><CC>001E; 001E01; 220</CC><FD>Analyse sensibilité; Traceur chimique; Transport; Modèle climat; Ozone; Troposphère; Mésosphère; Champ météorologique; Atmosphère; Prévision météorologique; Réanalyse; Méthane; Vapeur eau; Azote minéral; Climatologie; Satellite; Age; Air; In situ; Vent; Température; Simulation; Stratosphère; Oscillation quasi biennale; Circulation</FD><ED>sensitivity analysis; chemical tracers; transport; Climate models; ozone; troposphere; Mesosphere; Meteorological field; atmosphere; Weather forecast; Reanalysis; methane; water vapor; Inorganic nitrogen; Climatology; satellites; age; air; in situ; winds; temperature; simulation; stratosphere; Quasi biennial oscillation; circulation</ED><SD>Transporte; Ozono; Mesosfera; Campo meteorológico; Atmósfera; Predicción meteorológica; Reánalisis; Metano; Vapor agua; Nitrógeno inorgánico; Climatología; Satélite; Edad; Viento; Temperatura; Simulación; Estratosfera; Oscilación cuasi bienal</SD><LO>INIST-3144.354000173593090370</LO><ID>08-0011558</ID></server></inist></record>Pour manipuler ce document sous Unix (Dilib)
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